Photo-induced proton coupled electron transfer from a benzophenone 'antenna' to an isoindoline nitroxide
Morris, Jason C., Walsh, Liam, A., Gomes, Brunell A., Gigmes, Didier, Fairfull-Smith, Kathryn E., Bottle, Steven E., & Blinco, James P. (2015) Photo-induced proton coupled electron transfer from a benzophenone 'antenna' to an isoindoline nitroxide. RSC Advances, 5(116), pp. 95598-95603.
The current study reports the synthesis and properties of a novel isoindoline nitroxide contg. a benzophenone chromophore fused into the carbon framework. When exposed to UV light, rather than undergoing traditional benzophenone photochem. pathways, the presence of the nitroxide enables an energy transfer process whereby the nitroxide enters an excited state which induces an efficient hydrogen atom transfer from unactivated alkanes.
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|Item Type:||Journal Article|
|Divisions:||Current > Schools > School of Chemistry, Physics & Mechanical Engineering
Current > QUT Faculties and Divisions > Science & Engineering Faculty
|Deposited On:||23 Nov 2015 02:02|
|Last Modified:||24 Nov 2015 00:00|
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