Defect graphene as a trifunctional catalyst for electrochemical reactions

Jia, Yi, Zhang, Longzhou, Du, Aijun, Gao, Guoping, Chen, Jun, Yan, Xuecheng, Brown, Christopher L., & Yao, Xiangdong (2016) Defect graphene as a trifunctional catalyst for electrochemical reactions. Advanced Materials. (In Press)

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The defects derived by the removal of heteroatoms from graphene have been demonstrated, both experimentally and theoretically, to be effective for all three basic electrochemical reactions, e.g., oxygen reduction (ORR), oxygen evolution (OER), hydrogen evolution (HER). Density function theory calculations further reveal that the different types of defects are essential for the individual electrocatalytic activity for ORR, OER, and HER, respectively.

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ID Code: 98829
Item Type: Journal Article
Refereed: Yes
Keywords: defects; electrocatalysts; graphene; hydrogen evolution; oxygen reduction, oxygen evolution
DOI: 10.1002/adma.201602912
ISSN: 0935-9648
Divisions: Current > Schools > School of Chemistry, Physics & Mechanical Engineering
Current > QUT Faculties and Divisions > Science & Engineering Faculty
Copyright Owner: Copyright 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
Deposited On: 14 Sep 2016 22:48
Last Modified: 15 Sep 2016 21:59

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