Miktoarm star polymers via cyclodextrin-driven supramolecular self-assembly

Schmidt, B. V. K. J., Hetzer, M., Ritter, H., & Barner-Kowollik, C. (2012) Miktoarm star polymers via cyclodextrin-driven supramolecular self-assembly. Polymer Chemistry, 3(11).

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We report the formation of a novel class of supramolecular miktoarm star polymers via cyclodextrin host-guest chemistry. Reversible addition- fragmentation chain transfer polymerization from difunctional guest- or alkyne-containing chain transfer agents and copper(i)-catalyzed azide-alkyne cycloaddition leads to host- and guest-containing acrylamido polymers, namely poly(N,N-dimethylacrylamide) and poly(N,N-diethylacrylamide). Subsequently, a supramolecular miktoarm star polymer was formed and characterized via dynamic light scattering and rotating frame nuclear Overhauser effect spectroscopy. © 2012 The Royal Society of Chemistry.

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ID Code: 99322
Item Type: Journal Article
Refereed: Yes
Additional Information: Cited By :36 Export Date: 5 September 2016 Correspondence Address: Ritter, H.; Lehrstuhl für Präparative Polymerchemie, Institut für Organische Chemie und Makromolekulare Chemie, Heinrich-Heine Universität, Universitätsstrasse 1, Geb. 26.33.00, 40225 Düsseldorf, Germany; email: h.ritter@uni-duesseldorf.de References: Zayed, J.M., Nouvel, N., Rauwald, U., Scherman, O.A., (2010) Chem. Soc. Rev., 39, pp. 2806-2816; Altintas, O., Tunca, U., Barner-Kowollik, C., (2011) Polym. Chem., 2, pp. 1146-1155; Chen, S., Bertrand, A., Chang, X., Alcouffe, P., Ladavière, C., Gérard, J.-F., Lortie, F.R., Bernard, J., (2010) Macromolecules, 43, pp. 5981-5988; Fustin, C.A., Guillet, P., Schubert, U.S., Gohy, J.F., (2007) Adv. Mater., 19, pp. 1665-1673; Rauwald, U., Scherman, O.A., (2008) Angew. Chem., Int. Ed., 47, pp. 3950-3953; Yhaya, F., Lim, J., Kim, Y., Liang, M., Gregory, A.M., Stenzel, M.H., (2011) Macromolecules, 44, pp. 8433-8445; Köllisch, H.S., Barner-Kowollik, C., Ritter, H., (2009) Chem. Commun., pp. 1097-1099; Schmidt, B.V.K.J., Hetzer, M., Ritter, H., Barner-Kowollik, C., (2011) Macromolecules, 44, pp. 7220-7232; Chen, G., Jiang, M., (2011) Chem. Soc. Rev., 40, pp. 2254-2266; Stadermann, J., Komber, H., Erber, M., Däbritz, F., Ritter, H., Voit, B., (2011) Macromolecules, 44, pp. 3250-3259; Zeng, J., Shi, K., Zhang, Y., Sun, X., Zhang, B., (2008) Chem. Commun., pp. 3753-3755; Yan, Q., Xin, Y., Zhou, R., Yin, Y., Yuan, J., (2011) Chem. Commun., 47, pp. 9594-9596; Yan, Q., Yuan, J., Cai, Z., Xin, Y., Kang, Y., Yin, Y., (2010) J. Am. Chem. Soc., 132, pp. 9268-9270; Liu, H., Zhang, Y., Hu, J., Li, C., Liu, S., (2009) Macromol. Chem. Phys., 210, pp. 2125-2137; Kretschmann, O., Choi, S.W., Miyauchi, M., Tomatsu, I., Harada, A., Ritter, H., (2006) Angew. Chem., Int. Ed., 45, pp. 4361-4365; Nakahata, M., Takashima, Y., Yamaguchi, H., Harada, A., (2011) Nat. Commun., 2, p. 511; Schmidt, B.V.K.J., Rudolph, T., Hetzer, M., Ritter, H., Schacher, F.H., Barner-Kowollik, C., (2012) Polym. Chem., , 10.1039/c2py20293j; Zhang, Z.-X., Liu, X., Xu, F.J., Loh, X.J., Kang, E.-T., Neoh, K.-G., Li, J., (2008) Macromolecules, 41, pp. 5967-5970; Zhang, Z.-X., Liu, K.L., Li, J., (2011) Macromolecules, 44, pp. 1182-1193; Zhao, Q., Wang, S., Cheng, X., Yam, R.C.M., Kong, D., Li, R.K.Y., (2010) Biomacromolecules, 11, pp. 1364-1369; Bertrand, A., Stenzel, M., Fleury, E., Bernard, J., (2012) Polym. Chem., 3, pp. 377-383; Chiefari, J., Chong, Y.K., Ercole, F., Krstina, J., Jeffery, J., Le, T.P.T., Mayadunne, R.T.A., Thang, S.H., (1998) Macromolecules, 31, pp. 5559-5562; Barner-Kowollik, C., (2008) Handbook of RAFT-Polymerization, , ed., Wiley-VCH, Weinheim, Germany; Rekharsky, M.V., Inoue, Y., (1998) Chem. Rev., 98, pp. 1875-1918; Bigot, J., Charleux, B., Cooke, G., Delattre, Fo., Fournier, D., Lyskawa, Jl., Sambe, Ln., Woisel, P., (2010) J. Am. Chem. Soc., 132, pp. 10796-10801; Li, L.-Y., He, W.-D., Li, J., Zhang, B.-Y., Pan, T.-T., Sun, X.-L., Ding, Z.-L., (2010) Biomacromolecules, 11, pp. 1882-1890; Sakai, F., Chen, G., Jiang, M., (2012) Polym. Chem., 3, pp. 954-961
Keywords: Azide-alkyne cycloaddition, Chain transfer agents, Difunctional, Hostguest chemistry, Miktoarm star polymers, Poly(N , N-diethylacrylamide), Poly(N ,N-dimethylacrylamide), Reversible addition-fragmentation chain transfer, Rotating frame nuclear Overhauser effect spectroscopy, Supramolecular self-assemblies, Acetylene, Supramolecular chemistry, Polymers
DOI: 10.1039/c2py20214j
ISSN: 17599954
Divisions: Current > Schools > School of Chemistry, Physics & Mechanical Engineering
Current > Institutes > Institute for Future Environments
Current > QUT Faculties and Divisions > Science & Engineering Faculty
Deposited On: 22 Sep 2016 04:50
Last Modified: 05 Oct 2016 00:05

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